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第934回分子研コロキウム

演 題 「THz-APRES band structure movies of Dirac surface currents」
日 時 2019年11月12日(火) 16:00
講演者 Ulrich Höfer 教授(Department of Physics, Philipps-University of Marburg, Germany)
場 所

分子科学研究所 研究棟201

概 要

Time-resolved photoelectron spectroscopy combines femtosecond pump-probe techniques with angle-resolved photoelectron spectroscopy (ARPES). New opportunities for this powerful technique arise in combination with THz excitation. As an example, I will explain how THz-ARPES can be used to measure electron transport in the Dirac surface state of a three-dimensional topological insulator in a contact-free fashion and with femtosecond time-resolution. We induce electrical currents in these states with strong THz transients and directly access their dynamics in momentum space with subcycle time resolution. As a result of spin-momentum locking, the accelerated spin-polarized electrons reach ballistic mean free paths of several hundreds of nanometers. Topological insulators are thus promising materials for future lightwave- driven electronics [1].
Future applications of subcycle THz-ARPES are expected to benefit from the availability of high laser harmonics lab sources for photoemission or from combined THz + UV beamlines at synchrotrons or FELs. THz-ARPES of adsorbed molecules at surfaces should, e.g., make it possible to perform orbital tomography during chemical reactions.

[1] J. Reimann et al., Nature 562, 396 (2018).
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所内対応者:椴山儀恵、小林玄器(2019年度コロキウム委員)